Distributed Feedback Lasers by Thermal Nanoimprint of Perovskites Using Gelatin Gratings
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http://hdl.handle.net/10045/131782
Título: | Distributed Feedback Lasers by Thermal Nanoimprint of Perovskites Using Gelatin Gratings |
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Autor/es: | Allegro, Isabel | Bonal, Víctor | Mamleyev, Emil R. | Villalvilla, José M. | Quintana, José A. | Jin, Qihao | Díaz-García, María A. | Lemmer, Uli |
Grupo/s de investigación o GITE: | Física de la Materia Condensada |
Centro, Departamento o Servicio: | Universidad de Alicante. Departamento de Física Aplicada | Universidad de Alicante. Departamento de Óptica, Farmacología y Anatomía | Universidad de Alicante. Instituto Universitario de Materiales |
Palabras clave: | Nanoimprint lithography | Distributed feedback lasers | Perovskite films | Polymer gratings |
Fecha de publicación: | 31-ene-2023 |
Editor: | American Chemical Society |
Cita bibliográfica: | ACS Applied Materials & Interfaces. 2023, 15(6): 8436-8445. https://doi.org/10.1021/acsami.2c22920 |
Resumen: | To date, thermal nanoimprint lithography (NIL) for patterning hybrid perovskites has always involved an intricate etching step of a hard stamp material or its master. Here, we demonstrate for the first time the successful nanopatterning of a perovskite film by NIL with a low-cost polymeric stamp. The stamp consists of a dichromated gelatin grating structured by holographic lithography. The one-dimensional grating is imprinted into a perovskite film at 95 °C and 90 MPa for 10 min, resulting in a high quality second-order distributed feedback (DFB) laser. The laser exhibits an excellent performance with a threshold of 81 μJ/cm2, a line width of 0.32 nm, and a pronounced linear polarization. This novel approach enables cost-effective fabrication of high-quality DFB lasers compatible with different perovskite compositions and photonic nanostructures for a wide range of applications. |
Patrocinador/es: | We acknowledge the support of the Karlsruhe School of Optics & Photonics (KSOP) financed by the Ministry of Science, Research and the Arts of Baden-Wrttemberg as part of the sustainability financing of the projects of the Excellence Initiative II. We also acknowledge financial support through Germany’s Excellence Strategy via the Excellence Cluster 3D Matter Made to Order (3DMM2O, EXC-2082/1-390761711) and the Karlsruhe Nano Micro Facility (KNMFi). The group at the University of Alicante acknowledges financial support from the “Ministerio de Ciencia e Innovación/Agencia Estatal de Investigación” (MCIN/AEI) of Spain, the European Regional Development Fund, European Social Funds (project PID2020-106114GBI00), and the Conselleria de Innovación, Universidades y Sociedad Digital de la Comunidad Valenciana (Grant No. AICO/2021/093). V.B. acknowledges financial support from the University of Alicante to perform a research stay at KIT in the frame of his PhD. |
URI: | http://hdl.handle.net/10045/131782 |
ISSN: | 1944-8244 (Print) | 1944-8252 (Online) |
DOI: | 10.1021/acsami.2c22920 |
Idioma: | eng |
Tipo: | info:eu-repo/semantics/article |
Derechos: | © 2023 The Authors. Published by American Chemical Society |
Revisión científica: | si |
Versión del editor: | https://doi.org/10.1021/acsami.2c22920 |
Aparece en las colecciones: | INV - Física de la Materia Condensada - Artículos de Revistas |
Archivos en este ítem:
Archivo | Descripción | Tamaño | Formato | |
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Allegro_etal_2023_ACSApplMaterInterfaces_final.pdf | Versión final (acceso restringido) | 6,19 MB | Adobe PDF | Abrir Solicitar una copia |
Allegro_etal_2023_ACSApplMaterInterfaces_preprint.pdf | Preprint (acceso abierto) | 4,21 MB | Adobe PDF | Abrir Vista previa |
Allegro_etal_2023_ACSApplMaterInterfaces_supporting-information.pdf | Supporting Information | 751,38 kB | Adobe PDF | Abrir Vista previa |
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