Total oxidation of naphthalene at low temperatures using palladium nanoparticles supported on inorganic oxide-coated cordierite honeycomb monoliths

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dc.contributorMateriales Carbonosos y Medio Ambientees
dc.contributor.authorVarela Gandía, Francisco José-
dc.contributor.authorBerenguer-Murcia, Ángel-
dc.contributor.authorLozano Castelló, Dolores-
dc.contributor.authorCazorla-Amorós, Diego-
dc.contributor.authorSellick, David R.-
dc.contributor.authorTaylor, Stuart H.-
dc.contributor.otherUniversidad de Alicante. Departamento de Química Inorgánicaes
dc.contributor.otherUniversidad de Alicante. Instituto Universitario de Materialeses
dc.identifier.citationCatalysis Science & Technology. 2013, 3: 2708-2716. doi:10.1039/C3CY00323Jes
dc.identifier.issn2044-4753 (Print)-
dc.identifier.issn2044-4761 (Online)-
dc.description.abstractA study on the preparation of thin films of ZSM-5 and BETA zeolites, and a SAPO-5 silicoaluminophosphate, supported on cordierite honeycomb monoliths by in situ synthesis was carried out for their use as catalyst supports. Furthermore γ-Al2O3 was also coated onto a cordierite honeycomb monolith by a dip-coating method for use as a standard support. Structured monolithic catalysts were prepared by impregnation of the aforementioned coated monoliths with polymer-protected Pd nanoparticles. The monolithic catalysts have been tested for the total oxidation of naphthalene (100 ppm, GHSV 1220 h−1). From the combined use of the zeolite with polymer-protected nanoparticles, enhanced catalytic properties have been found for the total abatement of naphthalene. The Pd/MBETA and Pd/MZSM-5 catalytic monoliths have shown excellent activity with a high degree of stability, even after undergoing accelerated ageing
dc.description.sponsorshipThe authors would like to thank the Spanish MINECO, Generalitat Valenciana, and FEDER (Projects CTQ2012-31762 and PROMETEO/2009/047) for financial support. F. J. Varela-Gandía thanks the University of Alicante for a PhD studentship. Á. Berenguer-Murcia thanks the Spanish Ministry for Economy and Competitiveness for a Ramón y Cajal fellowship (RyC 2009-03913).es
dc.publisherRoyal Society of Chemistryes
dc.rights© The Royal Society of Chemistryes
dc.subjectPalladium nanoparticleses
dc.subjectCordierite honeycomb monolithses
dc.subject.otherQuímica Inorgánicaes
dc.titleTotal oxidation of naphthalene at low temperatures using palladium nanoparticles supported on inorganic oxide-coated cordierite honeycomb monolithses
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