Improved performance of perylenediimide-based lasers

Please use this identifier to cite or link to this item: http://hdl.handle.net/10045/38792
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dc.contributorFísica de la Materia Condensadaes
dc.contributor.authorGutiérrez Ramírez, Manuel-
dc.contributor.authorMorales-Vidal, Marta-
dc.contributor.authorNavarro-Fuster, Víctor-
dc.contributor.authorBoj Giménez, Pedro-
dc.contributor.authorQuintana Arévalo, José Antonio-
dc.contributor.authorVillalvilla Soria, José Moisés-
dc.contributor.authorRetolaza, Aritz-
dc.contributor.authorMerino, Santos-
dc.contributor.authorDíaz-García, María A.-
dc.contributor.otherUniversidad de Alicante. Departamento de Física Aplicadaes
dc.contributor.otherUniversidad de Alicante. Departamento de Óptica, Farmacología y Anatomíaes
dc.contributor.otherUniversidad de Alicante. Instituto Universitario de Materialeses
dc.date.accessioned2014-07-09T11:40:49Z-
dc.date.available2014-07-09T11:40:49Z-
dc.date.issued2013-02-14-
dc.identifier.citationJournal of Materials Chemistry C. 2013, 1: 1182-1191. doi:10.1039/C2TC00383Jes
dc.identifier.issn2050-7526 (Print)-
dc.identifier.issn2050-7534 (Online)-
dc.identifier.urihttp://hdl.handle.net/10045/38792-
dc.description.abstractThe aim of this work was to improve the laser performance, in terms of threshold and operational lifetime, of lasers based on polymer films doped with perylenediimide (PDI) derivatives as active media. For such purpose, we first investigated the amplified spontaneous emission (ASE) properties of perylene orange (PDI-O), when doped into polystyrene (PS) films. Lower ASE thresholds and larger photostabilities than those of similar films containing another PDI derivative (PDI-C6), recently reported in the literature, have been measured. Results have been interpreted in terms of the photoluminescence efficiency of the films, which depends on the type of molecular arrangement, inferred with the help of nuclear magnetic resonance experiments. We also show that PS films have a better ASE performance, i.e. lower thresholds and larger photostabilities, than those based on poly(methyl methacrylate), which was recently highlighted as one of the best matrixes for PDI-O. Finally, a one-dimensional second-order distributed feedback laser using PS doped with PDI-O was fabricated and characterized. This device has shown a threshold significantly lower (by around one order of magnitude) than that of a similar laser based on PDI-C6-doped PS.es
dc.description.sponsorshipWe thank support from the Spanish Government (MECC) and the European Community (FEDER) through grants MAT2008-06648-C02 and MAT-2011-28167-C02, as well as from the University of Alicante. MGR and MM are supported respectively by a CSIC fellowship within the program JAE and by MEC through a FPI fellowship.es
dc.languageenges
dc.publisherRoyal Society of Chemistryes
dc.rights© Royal Society of Chemistry 2014es
dc.subjectLaser performancees
dc.subjectPerylenediimide-based laserses
dc.subjectPDI-Oes
dc.subjectPDI-C6es
dc.subject.otherFísica Aplicadaes
dc.subject.otherÓpticaes
dc.subject.otherFísica de la Materia Condensadaes
dc.titleImproved performance of perylenediimide-based laserses
dc.typeinfo:eu-repo/semantics/articlees
dc.peerreviewedsies
dc.identifier.doi10.1039/C2TC00383J-
dc.relation.publisherversionhttp://dx.doi.org/10.1039/C2TC00383Jes
dc.rights.accessRightsinfo:eu-repo/semantics/openAccesses
Appears in Collections:INV - Física de la Materia Condensada - Artículos de Revistas
INV - GHPO - Artículos de Revistas

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