Improved performance of perylenediimide-based lasers

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Títol: Improved performance of perylenediimide-based lasers
Autors: Gutiérrez Ramírez, Manuel | Morales-Vidal, Marta | Navarro-Fuster, Víctor | Boj Giménez, Pedro | Quintana Arévalo, José Antonio | Villalvilla Soria, José Moisés | Retolaza, Aritz | Merino, Santos | Díaz-García, María A.
Grups d'investigació o GITE: Física de la Materia Condensada
Centre, Departament o Servei: Universidad de Alicante. Departamento de Física Aplicada | Universidad de Alicante. Departamento de Óptica, Farmacología y Anatomía | Universidad de Alicante. Instituto Universitario de Materiales
Paraules clau: Laser performance | Perylenediimide-based lasers | PDI-O | PDI-C6
Àrees de coneixement: Física Aplicada | Óptica | Física de la Materia Condensada
Data de publicació: 14-de febrer-2013
Editor: Royal Society of Chemistry
Citació bibliogràfica: Journal of Materials Chemistry C. 2013, 1: 1182-1191. doi:10.1039/C2TC00383J
Resum: The aim of this work was to improve the laser performance, in terms of threshold and operational lifetime, of lasers based on polymer films doped with perylenediimide (PDI) derivatives as active media. For such purpose, we first investigated the amplified spontaneous emission (ASE) properties of perylene orange (PDI-O), when doped into polystyrene (PS) films. Lower ASE thresholds and larger photostabilities than those of similar films containing another PDI derivative (PDI-C6), recently reported in the literature, have been measured. Results have been interpreted in terms of the photoluminescence efficiency of the films, which depends on the type of molecular arrangement, inferred with the help of nuclear magnetic resonance experiments. We also show that PS films have a better ASE performance, i.e. lower thresholds and larger photostabilities, than those based on poly(methyl methacrylate), which was recently highlighted as one of the best matrixes for PDI-O. Finally, a one-dimensional second-order distributed feedback laser using PS doped with PDI-O was fabricated and characterized. This device has shown a threshold significantly lower (by around one order of magnitude) than that of a similar laser based on PDI-C6-doped PS.
Patrocinadors: We thank support from the Spanish Government (MECC) and the European Community (FEDER) through grants MAT2008-06648-C02 and MAT-2011-28167-C02, as well as from the University of Alicante. MGR and MM are supported respectively by a CSIC fellowship within the program JAE and by MEC through a FPI fellowship.
URI: http://hdl.handle.net/10045/38792
ISSN: 2050-7526 (Print) | 2050-7534 (Online)
DOI: 10.1039/C2TC00383J
Idioma: eng
Tipus: info:eu-repo/semantics/article
Drets: © Royal Society of Chemistry 2014
Revisió científica: si
Versió de l'editor: http://dx.doi.org/10.1039/C2TC00383J
Apareix a la col·lecció: INV - Física de la Materia Condensada - Artículos de Revistas
INV - GHPO - Artículos de Revistas

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