Solution-processed nanographene distributed feedback lasers

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Title: Solution-processed nanographene distributed feedback lasers
Authors: Bonal, Víctor | Muñoz-Mármol, Rafael | Gordillo Gámez, Fernando | Morales-Vidal, Marta | Villalvilla Soria, José Moisés | Boj Giménez, Pedro | Quintana Arévalo, José Antonio | Gu, Yanwei | Wu, Jishan | Casado, Juan | Díaz-García, María A.
Research Group/s: Física de la Materia Condensada
Center, Department or Service: Universidad de Alicante. Departamento de Física Aplicada | Universidad de Alicante. Departamento de Óptica, Farmacología y Anatomía | Universidad de Alicante. Instituto Universitario de Materiales
Keywords: Nanographene | Distributed feedback lasers
Knowledge Area: Física Aplicada | Óptica | Física de la Materia Condensada
Issue Date: 25-Jul-2019
Publisher: Springer Nature
Citation: Nature Communications. 2019, 10: 3327. doi:10.1038/s41467-019-11336-0
Abstract: The chemical synthesis of nanographene molecules constitutes the bottom-up approach toward graphene, simultaneously providing rational chemical design, structure-property control and exploitation of their semiconducting and luminescence properties. Here, we report nanographene-based lasers from three zigzag-edged polycyclic aromatics. The devices consist of a passive polymer film hosting the nanographenes and a top-layer polymeric distributed feedback resonator. Both the active material and the laser resonator are processed from solution, key for the purpose of obtaining low-cost devices with mechanical flexibility. The prepared lasers show narrow linewidth ( < 0.13 nm) emission at different spectral regions covering a large segment of the visible spectrum, and up to the vicinity of the near-infrared. They show outstandingly long operational lifetimes (above 105 pump pulses) and very low thresholds. These results represent a significant step forward in the field of graphene and broaden its versatility in low-cost devices implying light emission, such as lasers.
Sponsor: The Alicante team acknowledges support from the Spanish Government (MINECO) and the European Community (FEDER) through grant no. MAT2015-66586-R. The researcher R.M.-M. has been partly supported by a MINECO FPI fellowship (no. BES-2016-077681). The work at the University of Málaga is supported by MINECO FEDER project reference CTQ2015-69391. J.W. acknowledges financial support from the MOE Tier 3 program (MOE2014-T3-1-004) and NRF Investigatorship Award (NRF-NRFI05-2019-0005).
URI: http://hdl.handle.net/10045/94860
ISSN: 2041-1723
DOI: 10.1038/s41467-019-11336-0
Language: eng
Type: info:eu-repo/semantics/article
Rights: © The Author(s) 2019. Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
Peer Review: si
Publisher version: https://doi.org/10.1038/s41467-019-11336-0
Appears in Collections:INV - Física de la Materia Condensada - Artículos de Revistas

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