Plasma-Assisted Synthesis of Monodispersed and Robust Ruthenium Ultrafine Nanocatalysts for Organosilane Oxidation and Oxygen Evolution Reactions
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Título: | Plasma-Assisted Synthesis of Monodispersed and Robust Ruthenium Ultrafine Nanocatalysts for Organosilane Oxidation and Oxygen Evolution Reactions |
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Autor/es: | Gnanakumar, Edwin S. | Ng, Wesley | Filiz, Bilge Coşkuner | Rothenberg, Gadi | Wang, Sheng | Xu, Hualong | Pastor Pérez, Laura | Pastor-Blas, M. Mercedes | Sepúlveda-Escribano, Antonio | Yan, Ning | Shiju, N. Raveendran |
Grupo/s de investigación o GITE: | Materiales Avanzados |
Centro, Departamento o Servicio: | Universidad de Alicante. Departamento de Química Inorgánica | Universidad de Alicante. Instituto Universitario de Materiales |
Palabras clave: | Nanostructures | Oxidation | Plasma chemistry | Ruthenium | Supported catalysts |
Área/s de conocimiento: | Química Inorgánica |
Fecha de publicación: | 12-oct-2017 |
Editor: | Wiley-VCH Verlag GmbH & Co. KGaA |
Cita bibliográfica: | ChemCatChem. 2017, 9(22): 4159-4163. doi:10.1002/cctc.201700809 |
Resumen: | We report a facile and general approach for preparing ultrafine ruthenium nanocatalysts by using a plasma-assisted synthesis at <100 °C. The resulting Ru nanoparticles are monodispersed (typical size 2 nm) and remain that way upon loading onto carbon and TiO2 supports. This gives robust catalysts with excellent activities in both organosilane oxidation and the oxygen evolution reaction. |
Patrocinador/es: | N.R.S. and E.S.G. acknowledge financial support from the NOW CAPITA project (732.013.002). A.S.E. acknowledges financial support from Generalitat Valenciana, Spain (Project PROMETEOII/2014/004). This work is part of the Research Priority Area Sustainable Chemistry of the University of Amsterdam, http://suschem.uva.nl |
URI: | http://hdl.handle.net/10045/70269 |
ISSN: | 1867-3880 (Print) | 1867-3899 (Online) |
DOI: | 10.1002/cctc.201700809 |
Idioma: | eng |
Tipo: | info:eu-repo/semantics/article |
Derechos: | © 2017 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA. This is an open access article under the terms of the Creative Commons Attribution-NonCommercial License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited and is not used for commercial purposes. |
Revisión científica: | si |
Versión del editor: | http://dx.doi.org/10.1002/cctc.201700809 |
Aparece en las colecciones: | INV - LMA - Artículos de Revistas |
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