An Efficient and Color-Tunable Solution-Processed Organic Thin-Film Laser with a Polymeric Top-Layer Resonator

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Title: An Efficient and Color-Tunable Solution-Processed Organic Thin-Film Laser with a Polymeric Top-Layer Resonator
Authors: Quintana Arévalo, José Antonio | Villalvilla Soria, José Moisés | Morales-Vidal, Marta | Boj Giménez, Pedro | Zhu, Xiaozhang | Ruangsupapichat, Nopporn | Tsuji, Hayato | Nakamura, Eiichi | Díaz-García, María A.
Research Group/s: Física de la Materia Condensada
Center, Department or Service: Universidad de Alicante. Departamento de Física Aplicada | Universidad de Alicante. Departamento de Óptica, Farmacología y Anatomía | Universidad de Alicante. Instituto Universitario de Materiales
Keywords: Distributed feedback lasers | Organic lasers | Polymeric resonators | Solution-processed
Knowledge Area: Física Aplicada | Óptica | Física de la Materia Condensada
Issue Date: 2-Oct-2017
Publisher: Wiley-VCH Verlag GmbH & Co. KGaA
Citation: Advanced Optical Materials. 2017, 5(19): 1700238. doi:10.1002/adom.201700238
Abstract: Thin film organic lasers represent attractive light sources for numerous applications. Currently, efforts are devoted to the development of low-cost high-performance and color-tunable devices, whereby both the resonator and the active layer should consist of solution-processable organic materials. Herein, solution-processed distributed-feedback lasers are reported with polymeric resonators on top of active films of perylene orange or carbon-bridged oligo(p-phenylenevinylene) dispersed in polystyrene, which combine these properties. These lasers emit in the 520–595 nm range and show low thresholds (≈1 kW cm−2) and long operational lifetimes (7 × 105 pump pulses), which are comparable to other state-of-the-art lasers that contain the same active materials but resonators made on inorganic substrates. Due to this top-layer resonator configuration, the laser slope efficiencies of the present devices are remarkably superior. A centimeter-size device emitting at different wavelengths within a broad spectral range, based on a perylene-based film of uniform thickness that contributes to preserve a low threshold, is demonstrated.
Sponsor: The Spanish team acknowledges support from the Spanish Government (MINECO) and the European Community (FEDER) through Grant Nos. MAT2011-28167-C02-01 and MAT2015-66586-R. M.M.-V. was partly supported by a MINECO FPI fellowship (No. BES-2009-020747) and by a Junta de Castilla y León grant (No. SA046U16). Japanese authors thank the financial support from the MEXT (16H04106 for H.T. and 15H05754 for E.N.).
URI: http://hdl.handle.net/10045/69931
ISSN: 2195-1071
DOI: 10.1002/adom.201700238
Language: eng
Type: info:eu-repo/semantics/article
Rights: © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
Peer Review: si
Publisher version: http://dx.doi.org/10.1002/adom.201700238
Appears in Collections:INV - Física de la Materia Condensada - Artículos de Revistas
INV - GHPO - Artículos de Revistas

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